Optimizing radiolabeled engineered anti-p185HER2 antibody fragments for in vivo imaging

Cancer Res. 2005 Jul 1;65(13):5907-16. doi: 10.1158/0008-5472.CAN-04-4472.

Abstract

We have recently described the in vivo properties of an iodinated anti-p185HER2 engineered antibody fragment [minibody (scFv-C(H)3)2; 80 kDa], made from the internalizing 10H8 monoclonal antibody. Although the 10H8 minibody showed excellent binding to the target in vitro, only modest tumor uptake [5.6 +/- 1.7% injected dose per gram (ID/g) of tissue] was achieved in nude mice bearing MCF7/HER2 breast cancer tumors. Here, in an attempt to improve targeting, the 10H8 minibody was conjugated to 1,4,7,10-tetraazacyclododecane-N, N', N'', N'''-tetraacetic acid (DOTA), radiometal labeled, and evaluated in vivo. The tumor uptake of 111In-DOTA 10H8 minibody was 5.7 +/- 0.1% ID/g, similar to the radioiodinated 10H8 minibody. However, in addition to the expected liver clearance, the kidneys had unexpectedly high activity (34.0 +/- 4.0% ID/g). A minibody derived from a second anti-p185(HER2) antibody (trastuzumab; hu4D5v8) was also made. Tumor uptakes, evaluated by quantitative microPET using 64Cu-DOTA hu4D5v8 minibody, were 4.2 +/- 0.5% ID/g. Furthermore, in non-tumor-bearing mice, 111In-DOTA hu4D5v8 minibody exhibited similar elevated uptake in the kidneys (28.4 +/- 6.5% ID/g). Immunohistochemical staining of kidneys from non-tumor-bearing mice showed strong specific staining of the proximal tubules, and Western blot analysis of kidney lysate confirmed the presence of cross-reactive antigen. To further improve tumor uptake and normal tissue distribution, a larger hu4D5v8 fragment [(scFv-C(H)2-C(H)3)2; 105 kDa] was made, engineered to exhibit rapid clearance kinetics. This fragment, when evaluated by microPET, exhibited improved tumor targeting (12.2 +/- 2.4% ID/g) and reduced kidney uptake (13.1 +/- 1.5% ID/g). Thus, by manipulating the size and format of anti-p185(HER2) antibody fragments, the kidney activity was reduced and high or low expression of p185HER2 in xenografts could be distinguished by microPET imaging.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Breast Neoplasms / diagnostic imaging
  • Breast Neoplasms / immunology
  • Breast Neoplasms / metabolism
  • Carcinoembryonic Antigen / immunology
  • Copper Radioisotopes / pharmacokinetics
  • Female
  • Humans
  • Immunoconjugates / chemistry
  • Immunoconjugates / pharmacokinetics*
  • Immunoglobulin Fragments / chemistry
  • Immunoglobulin Fragments / metabolism*
  • Indium Radioisotopes / chemistry
  • Indium Radioisotopes / pharmacokinetics
  • Kidney / diagnostic imaging
  • Kidney / immunology
  • Kidney / metabolism
  • Mice
  • Mice, Nude
  • Neoplasms / diagnostic imaging*
  • Neoplasms / immunology
  • Neoplasms / metabolism
  • Positron-Emission Tomography
  • Radiopharmaceuticals / chemistry
  • Radiopharmaceuticals / pharmacokinetics
  • Receptor, ErbB-2 / chemistry
  • Receptor, ErbB-2 / immunology*
  • Receptor, ErbB-2 / metabolism
  • Tissue Distribution

Substances

  • Carcinoembryonic Antigen
  • Copper Radioisotopes
  • Immunoconjugates
  • Immunoglobulin Fragments
  • Indium Radioisotopes
  • Radiopharmaceuticals
  • Receptor, ErbB-2