Aldohexuronic acid catabolism by a soil Aeromonas

J Bacteriol. 1969 Jan;97(1):97-106. doi: 10.1128/jb.97.1.97-106.1969.

Abstract

Bacteria which utilize mannuronic acid as an energy source were isolated from nature. One of the organisms, identified as a member of the genus Aeromonas, used glucuronate, galacturonate, and mannuronate as the sole source of carbon and energy. Glucuronate- and galacturonate-grown resting cells oxidized both glucuronate and galacturonate rapidly, but mannuronate slowly. Mannuronate-grown cells oxidized all three rapidly, with the rate of mannuronate utilization somewhat lower. Cell-free extracts from glucuronate-, galacturonate-, and mannuronate-grown Aeromonas C11-2B contained glucuronate and galacturonate isomerases, fructuronate, tagaturonate, and mannuronate reductases, and mannonate and altronate dehydratases, with the exception of glucuronate-grown cells which lacked altronate dehydratase. Thus, the pathway for glucuronate and galacturonate catabolism for Aeromonas was identical to Escherichia coli. Glucuronate and galacturonate were isomerized to d-fructuronate and d-tagaturonate which were then reduced by reduced nicotinamide adenine dinucleotide to d-mannonate and d-altronate, respectively. The hexonic acids were dehydrated to 2-keto-3-deoxy gluconate which was phosphorylated by adenosine triphosphate to 2-keto-3-deoxy-6-phospho gluconate. The latter was then cleaved to pyruvate and glyceraldehyde-3-phosphate. Mannuronate was reduced directly to d-mannonate by a reduced nicotinamide adenine dinucleotide phosphate-linked oxidoreductase. d-Mannonate was then further broken down as in the glucuronate pathway. The mannuronate reducing enzyme, for which the name d-mannonate:nicotinamide adenine dinucleotide (phosphate) oxidoreductase (d-mannuronate-forming) was proposed, was shown to be distinct from altronate and mannoate oxidoreductases. This is the first report of a bacterial oxidoreductase which reduces an aldohexuronic acid to a hexonic acid. The enzyme should prove to be a useful analytical tool for determining mannuronate in the presence of other uronic acids.

MeSH terms

  • Aeromonas / metabolism*
  • Alcohol Oxidoreductases / metabolism
  • Fructose
  • Galactose / metabolism
  • Glucuronates
  • Glyceraldehyde / biosynthesis
  • Hydro-Lyases / metabolism
  • Isomerases / metabolism
  • Mannose / metabolism
  • NADP
  • Oxidoreductases / metabolism*
  • Phosphates / biosynthesis
  • Pyruvates / biosynthesis
  • Soil Microbiology*
  • Terminology as Topic
  • Uronic Acids / metabolism*

Substances

  • Glucuronates
  • Phosphates
  • Pyruvates
  • Uronic Acids
  • Fructose
  • Glyceraldehyde
  • NADP
  • Oxidoreductases
  • Alcohol Oxidoreductases
  • Hydro-Lyases
  • Isomerases
  • Mannose
  • Galactose